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1.
Stochastic resonance (SR) has been extensively utilized in the field of weak fault signal detection for its characteristic of enhancing weak signals by transferring the noise energy. Aiming at solving the output saturation problem of the classical bistable stochastic resonance (CBSR) system, a double Gaussian potential stochastic resonance (DGSR) system is proposed. Moreover, the output signal-to-noise ratio (SNR) of the DGSR method is derived based on the adiabatic approximation theory to analyze the effect of system parameters on the DGSR method. At the same time, for the purpose of overcoming the drawback that the traditional SNR index needs to know the fault characteristic frequency (FCF), the weighted local signal-to-noise ratio (WLSNR) index is constructed. The DGSR with WLSNR can obtain optimal parameters adaptively, thereby establishing the DGSR system. Ultimately, a DGSR method is proposed and applied in centrifugal fan blade crack detection. Through simulations and experiments, the effectiveness and superiority of the DGSR method are verified.  相似文献   
2.
氢能的引入能有效提升配电网的供电可靠性,而电解水制氢是实现低碳转型的关键技术,开发高效的电解水催化剂势在必行。过渡金属氧化物储量大、催化活性高,是具有广阔应用前景的析氧反应催化剂。本文通过射频等离子体处理制备石墨烯上负载Co3O4析氧催化剂,XRD、Raman和XPS测试结果显示,二维结构石墨烯的引入加速表面电子迁移,增大了反应面积。等离子体处理促进了纳米粒子在石墨烯上的负载,利用等离子体刻蚀作用在催化剂表面制造出大量碳结构缺陷和氧空位结构,改善了活性位点分布,有效调控Co3O4电子结构,提高析氧催化活性。电化学测试表明,本文中合成的Co3O4@rGO在电流密度为50 mA·cm-2时的过电位为410 mV,动力学反应速率较快,表现出优于商业IrO2的析氧催化活性。  相似文献   
3.
Archive of Applied Mechanics - Membranes are widely applied in the large-span buildings and spatial deployable structures. They are prone to wrinkle under compression due to their small bending...  相似文献   
4.
Shock testing is an important issue for the survivability of an equipment under shock environment in aerospace and military industries. One of the problems faced in conventional shock testing devices is the need for redesigning of the geometry whenever the responses to different shock environments are tested. To circumvent the redesigning processes, a structure with two ‘acoustic black holes (ABHs)’ on both ends, referred to as the beam with dual ABHs, is proposed as a shock testing device. The beam with dual ABHs is capable of simulating diverse shock environments by controlling the applied force because it can be regarded as an infinite beam at high frequency range with the aid of the anechoic terminations by the ABHs. To systematically investigate the beam with dual ABHs, we develop a wave-based method that uses the reflection matrix of an ABH to perform free and forced vibration analyses. From the analyses on frequency response function and shock response spectrum of the beam with dual ABH, it is suggested that the beam with dual ABHs is feasible as a semi-permanent shock testing device.  相似文献   
5.
Electrically conductive polypropylene/graphite (PP/graphite) composites were prepared via blending granulated PP with maleic anhydride grafted PP and natural graphite. Electrical conductivity of prepared samples containing either 65, 70, or 75 wt% of graphite was measured and the most conductive sample containing 75 wt% of graphite was exposed to UV irradiation for 1 and 24 h or thermally treated at 170 °C for 1 h. The influence of thermal and UV exposure on the structural and electrical changes in such treated samples was studied. Local current measurements on the surface were made using scanning spreading resistance microscopy and morphology of the surface was studied by atomic force microscopy. X-ray diffraction analysis, infrared and Raman spectroscopy were also used for the structural characterization. Properties of treated and untreated samples are compared and differences are discussed.  相似文献   
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7.
《中国化学快报》2020,31(6):1415-1421
Electrocatalytic CO_2 reduction(CO_2 ER) into formate is a desirable route to achieve efficient transformation of CO_2 to value-added chemicals,however,it still suffers from limited catalytic activity and poor selectivity.Herein,we develop a hybrid electrocatalyst composed of bismuth and bismuth oxide nanoparticles(NPs) supported on nitrogen-doped reduced graphene oxide(Bi/Bi_2 O_3/NrGO) nanosheets prepared by a combined hydrothermal with calcination treatment.Thanks to the combination of undercoordinated sites and strong synergistic effect between Bi and Bi_2 O_3,Bi/Bi_2 O_3/NrGO-700 hybrid displays a promoted CO2 ER catalytic performance and selectivity for formate production,as featured by a small onset potential of-0.5 V,a high current density of-18 mA/cm~2,the maximum Faradaic efficiency of85% at-0.9 V,and a low Tafel slope of 166 mV/dec.Experimental results reveal that the higher CO_2 ER performance of Bi/Bi_2 O_3/NrGO-700 than that of Bi NPs supported on NrGO(Bi/NrGO) can be due to the partial reduction of Bi_2 O_3 NPs into Bi,which significantly increases undercoordinated active sites on Bi NPs surface,thus boosting its CO_2 ER performance.Furthermore,a two-electrode device with Ir/C anode and Bi/Bi_2 O_3/NrGO-700 cathode could be integrated with two alkaline batteries or a planar solar cell to achieve highly active water splitting and CO_2 ER.  相似文献   
8.
Yao  Wen  Chen  Yangfan  Li  Jiangling  Yang  Jian  Ren  Shan  Liu  Weizao  Liu  Qingcai 《Research on Chemical Intermediates》2022,48(5):1813-1829
Research on Chemical Intermediates - Industrial wastewater is becoming a universal environmental problem, wherein toxic organic compounds are important sources of pollution. For the degradation...  相似文献   
9.
张颂  魏彪  刘易鑫  毛本将  钱易坤  黄宇晨  冯鹏 《强激光与粒子束》2020,32(5):056001-1-056001-7
研究用于校准场所中子剂量监测仪表的241Am-Be中子参考辐射场计量特性。采用蒙特卡罗方法模拟了空气自由中子参考辐射(FRNR),GB/T 14055规定的最小尺寸中子参考辐射(SRNR)和实际中子参考辐射(ARNR)中不同检验点处中子周围剂量当量率、散射中子占比和能谱分布特征。研究结果表明,空气对FRNR中的剂量率和能谱分布影响小,近似为理想中子参考辐射;采用5%含硼聚乙烯作屏蔽的最小尺寸SRNR可减少热中子,降低散射中子占比,影锥法不适用于小尺寸中子参考辐射中对散射中子的修正;ARNR中的散射中子更少、占比更低,影锥法所得散射中子占比与理论值基本一致。  相似文献   
10.
《中国化学快报》2020,31(6):1654-1659
The carbon quantum dots(CQDs) and their functionalized materials are promising in biomedical field because of their unique properties;meanwhile,a growing concern has been raised about the potential toxicity of these modified materials in biosystem.In this study,we synthesized original CQDs and two common functionalized CQDs including N-doped CQDs(NCQDs) and folic acid-modified CQDs(FACQDs),and compared the toxicity and biocompatibility with each other in vitro and in vivo.L929,C6 and normal cell MDCK were selected to detect the adverse reaction of these materials in vitro.No acute toxicity or obvious changes were noted from in vitro cytotoxicity studies with the dose of these CQD materials increasing to a high concentration at 1 mg/mL.Among these materials,the FA-CQDs show a much lower toxicity.Moreover,in vivo toxicity studies were performed on the nude mice for 15 days.The experimental animals in 10 or 15 mg/kg groups were similar with animals treated by phosphate buffer solution(PBS) after 15 days.The results of the multifa rious biochemical parameters also suggest that the functionalized products of CQDs do not influence the biological indicators at feasible concentration.Our findings in vitro and in vivo through toxicity tests demonstrate that CQDs and their modified materials are safe for future biological applications.  相似文献   
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